Discovery of 20028-53-9

Compounds in my other articles are similar to this one(2-Amino-5-chlorobenzaldehyde)SDS of cas: 20028-53-9, you can compare them to see their pros and cons in some ways,such as convenient, effective and so on.

In organic chemistry, atoms other than carbon and hydrogen are generally referred to as heteroatoms. The most common heteroatoms are nitrogen, oxygen and sulfur. Now I present to you an article called Regiodivergent Intramolecular Nucleophilic Addition of Ketimines for the Diverse Synthesis of Azacycles, published in 2020, which mentions a compound: 20028-53-9, mainly applied to indolyloxindole indoleacetate regioselective preparation; tetrahydrospiroquinolineoxindole regioselective diastereoselective enantioselective preparation; nitroethylaniline imine oxindole ketoester regioselective cyclization; sodium catalyst regioselective cyclization nitroethylaniline imine oxindole ketoester; copper catalyst stereoselective spirocyclization nitroethylaniline imine oxindole ketoester; transition state solvent effect regioselective cyclization nitroethylaniline imine oxindole; heterocycles; indoles; organocatalysis; reaction mechanisms; synthetic methods, SDS of cas: 20028-53-9.

Imines generated in situ or prepared from isatins or aryl α-ketoesters and 2-(2-nitroethyl)anilines underwent regioselective, diastereoselective, and enantioselective cyclization reactions to yield indolyloxindoles such as I and indoleacetates or tetrahydrospiroquinolineoxindoles such as II or tetrahydroquinolinecarboxylates. Cyclocondensation of oxindoles with 2-(2-nitroethyl)anilines in MeOH in the presence of p-TsOH followed by treatment with Na2CO3 in MeOH yielded indolyloxindoles such as I, while imines prepared from 2-(2-nitroethyl)anilines and α-ketoesters underwent cyclization in the presence of Na2CO3 and KHCO3 in MeOH to yield indoleacetates. In the presence of Cu(BF4)2 and a nonracemic bisoxazoline, imines prepared from isatins and 2-(2-nitroethyl)anilines underwent regioselective, diastereoselective, and enantioselective cyclization to yield tetrahydrospiroquinolineoxindoles. Selected products were further functionalized; I was converted in three steps to a nonracemic intermediate in the preparation of (-)-psychotrimine. Computational study of the mechanism and of the effect of solvent on the reaction regiochem. indicated that hydrogen-bonding interactions facilitate the nucleophilic attack of imines at the nitrogen atom.

Compounds in my other articles are similar to this one(2-Amino-5-chlorobenzaldehyde)SDS of cas: 20028-53-9, you can compare them to see their pros and cons in some ways,such as convenient, effective and so on.

Reference:
Tetrahydrofuran – Wikipedia,
Tetrahydrofuran | (CH2)3CH2O – PubChem